18–26 Sept 2025
Ito International Research Center
Asia/Tokyo timezone

Studies as a function of different ALD capping layers on cavity losses for QIS and accelerators

THA04
25 Sept 2025, 09:30
20m
Ito International Research Center

Ito International Research Center

Tokyo
Board: THA04
Invited Oral Presentation MC2: Fundamental SRF research and development Thursday Oral Session: A

Speaker

Laura Grassellino (Fermi National Accelerator Laboratory)

Description

Niobium-based bulk SRF cavities have demonstrated exceptional performance. To further improve niobium cavity performance, we present studies involving a novel surface engineering process designed to prevent the formation of amorphous niobium oxides on the surface. This is achieved by encapsulating the niobium surface using thermal Atomic-Layer-Deposition (ALD). This technique has been shown to enhance the properties of niobium cavities and 2D resonators. This study not only aims to improve SRF performance at high fields but also has the potential to enhance the quality factor in low-field regimes, particularly for quantum applications. For the method to be effective, it is essential to have a clean interface between the encapsulating layer and the bulk niobium. Achieving this requires a uniform coating across the entire cavity surface and efficient removal of the underlying niobium oxides. To optimize the process, a variety of material characterization tools have been utilized to refine parameters such as thin film thickness and annealing conditions. Cavity RF measurements were performed at the vertical test facilities at FNAL to assess the Q vs. Eacc curves for accelerator applications, as well as at the SQMS dilution refrigerators to investigate the full two-level system (TLS) losses at milliKelvin and single-photon levels. Based on the results, we characterized the loss of different oxides in various regimes and applications, comparing them to natural niobium pentoxide.

Funding Agency

This material is based upon work supported by the U.S. Department of Energy, Office of Science, National Quantum Information Science Research Centers, Superconducting Quantum Materials and Systems Cen

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Author

Laura Grassellino (Fermi National Accelerator Laboratory)

Co-authors

Akshay Murthy (Fermi National Accelerator Laboratory) Alexander Romanenko (Fermi National Accelerator Laboratory) Anna Grassellino (Fermi National Accelerator Laboratory) Daniel Bafia (Fermi National Accelerator Laboratory) Grigory Eremeev (Fermi National Accelerator Laboratory) Sam Posen (Fermi National Accelerator Laboratory) Sergey Belomestnykh (Fermi National Accelerator Laboratory) Thomas Proslier (Université Paris-Saclay) Yasmine Kalboussi (Commissariat à l'Energie Atomique)

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