Speaker
Description
X-ray free-electron lasers have opened new frontiers in attosecond science thanks to their high pulse energy compared to traditional table top sources. To date, most attosecond experiments performed at XFELs have been impulsive, with the impinging x-ray pulses being much shorter than the timescales being studied. We present a method for attosecond pulse shaping which enables us to move beyond simple observation of ultrafast dynamics towards coherent control of quantum systems on sub-femtosecond timescales. We present experimental evidence of phase locked attosecond pulse trains from the LCLS-II. We conclude by presenting recent experiments utilizing mutually coherent pulse pairs with controllable temporal and spectral delay to launch controllable coherent electronic wavepackets in molecular systems.
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